up::[[Combustion]]
https://www.youtube.com/watch?v=rUBXCn9TSas
We need to make the following assumptions to formulate the adiabatic flame temperature:
- Chemical reactions happen in gaseous state
- All gases are perfect gases
- "Calorically perfect gas" means [[Specific heat]]s $c_p$ and $c_v$ can be treated as constant instead of a function of temperature
- Chemical process occur between equilibrium states
## 1. Some intro
To generalize we write chemical reaction like this:
$\sum_{i=1}^{N}\ce{n_i^'m_i->}\sum_{i=1}^{N}\ce{n_i^{''}m_i}$
Note all reactants and products are on both sides.
[[Enthalpy of reaction]] is
$Q_p=\Delta H = H_{reactants}-H_{products}$
$\displaylines{Q_p = \sum_{i=1}^N n_i^{''}\left[{\Delta_{f}}_{STP}H^{\ominus} + \left(h_f(T)-h_{fSTP}^{\ominus}\right)\right]_{products}- \\
\sum_{i=1}^N n_i^{'}\left[{\Delta_{f}}_{STP}H^{\ominus} + \left(h_f(T)-h_{fSTP}^{\ominus}\right)\right]_{reactants}}$
if you set $Q_p=0$ (since it is adiabatic) which means $H_{reactants}=H_{products}$
If we assume pressure is also constant you can set the change in sensible enthalpy of the products to $c_p \Delta T$ and calculate the adiabatic flame temperature.
## 2. Adiabatic Flame temperature
In order for a reaction to produce high adiabatic flame temperature (i.e. combustion) i.e. the sensible enthalpy of the products $\left(h_f(T)-h_{fSTP}^{\ominus}\right)$ to be high:
- The standard enthalpy of the products needs to be a large negative value. i.e the combustion should produce reactants which are stable i.e. stoichiometric reaction
- The standard enthalpy of the reactants should be high
- especially the fuel if the oxidizer is oxygen
- The sensible enthalpy of the reactants is low (the reactants are at much lower temperature than the products)
## 3. Non-stoichiometric conditions
At non-stoichiometric conditions, excess fuel or oxidizer remains and it needs to be raised to the same temperature as the products (increase in sensible enthalpy). Hence non-stoichiometric reactions produce lower temperatures than stoichiometric reactions.
Note: fuels tend to have higher $c_p$ compared to oxidizers. hence the slope of the curve tends to be steeper on the fuel rich side compared to the oxygen rich side in this [[Mixture Ratio]] vs flame temperature curve
![[temp_vs_mr.png]]
Tools like NASA [[CEA]] and STANJAN can be used to calculate adiabatic flame temperature for various reactions.
## 4. Impact of Pressure
Pressure affects the composition of products of combustion (proportion of stable and unstable products) and hence affects the adiabatic flame temperature. This effect is generally small.
https://www.researchgate.net/publication/338157321_The_adiabatic_flame_temperature_and_laminar_flame_speed_of_methane_premixed_flames_at_varying_pressures